Anthropogenic Impacts on Tropospheric Reactive Chlorine Since the Preindustrial

نویسندگان

چکیده

Tropospheric reactive gaseous chlorine (Cly) impacts the atmosphere's oxidation capacity with implications for chemically reduced gases such as methane. Here we use Greenland ice-core records of chlorine, sodium, and acidity, global model simulations to show how tropospheric Cly has been impacted by anthropogenic emissions since 1940s. We that contribution nonsea-salt significantly influenced total its trends after The modeled regional 170% increase from preindustrial 1970s was driven acid displacement sea-salt-aerosol, direct emission hydrochloric (HCl) combustion, chemical reactions nitrogen oxide (NOx) emissions. Since 1970s, 6% decrease caused mainly HCl air pollution mitigation policies. Our findings suggest acidic their control strategies have substantial on oxidants, methane, mercury.

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ژورنال

عنوان ژورنال: Geophysical Research Letters

سال: 2021

ISSN: ['1944-8007', '0094-8276']

DOI: https://doi.org/10.1029/2021gl093808